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Transformation behaviors and environmental risk assessment of heavy metals during resource recovery from Sedum plumbizincicola via hydrothermal liquefaction

He Chao, Zhang Zhao, Xie Candie, Giannis Apostolos, Chen Zhe, Tang Yetao, Qiu Rongliang

Απλή Εγγραφή


URIhttp://purl.tuc.gr/dl/dias/D1282DC5-DD88-42D8-B968-E13A48D0F493-
Αναγνωριστικόhttps://doi.org/10.1016/j.jhazmat.2020.124588-
Αναγνωριστικόhttps://www.sciencedirect.com/science/article/pii/S0304389420325784-
Γλώσσαen-
Μέγεθος11 pagesen
ΤίτλοςTransformation behaviors and environmental risk assessment of heavy metals during resource recovery from Sedum plumbizincicola via hydrothermal liquefactionen
ΔημιουργόςHe Chaoen
ΔημιουργόςZhang Zhaoen
ΔημιουργόςXie Candieen
ΔημιουργόςGiannis Apostolosen
ΔημιουργόςΓιαννης Αποστολοςel
ΔημιουργόςChen Zheen
ΔημιουργόςTang Yetaoen
ΔημιουργόςQiu Rongliangen
ΕκδότηςElsevieren
ΠερίληψηEnvironmentally sound disposal of hyperaccumulator harvests is of critical importance to industrialization of phytoremediation. Herein, transformation behaviors and environmental risk of heavy metals were comprehensively examined during subcritical hydrothermal liquefaction of Sedum plumbizincicola. It is concluded that low temperature liquefaction favored resource recovery of heavy oil and hydrochars in terms of higher energy density, improved carbon sequestration and less energy consumption. Heavy metals were mainly distributed into hydrochars and water soluble phase with less than 10% in heavy oil. All metal elements except As could be accumulated in hydrochars by extending reaction time, whereas more than 96% of As was redistributed into water soluble phase. Prolonged liquefaction time facilitated immobilization of Cd, Cr and As in hydrochars, but fast liquefaction favored Pb stabilization. Liquefaction significantly reduced environmental risk level of Cd, Zn and As, but may mobilize Pb and Mn, especially for Mn to very high risk level at 240 ºC. High temperature with long reaction time tended to inhibit leaching rate of Mn, whereas low liquefaction temperature with short reaction time prevented the leaching of Zn and As from hydrochars. Overall, these findings are essential for downstream upgrading of heavy oil and metals recovery from hydrochars.en
ΤύποςPeer-Reviewed Journal Publicationen
ΤύποςΔημοσίευση σε Περιοδικό με Κριτέςel
Άδεια Χρήσηςhttp://creativecommons.org/licenses/by/4.0/en
Ημερομηνία2022-04-19-
Ημερομηνία Δημοσίευσης2020-
Θεματική ΚατηγορίαPhytoremediationen
Θεματική ΚατηγορίαHyperaccumulatoren
Θεματική ΚατηγορίαHeavy oilen
Θεματική ΚατηγορίαHydrocharen
Θεματική ΚατηγορίαRACen
Βιβλιογραφική ΑναφοράC. He, Z. Zhang, C. Xie, A. Giannis, Z. Chen, Y. Tang, and R. Qiu, “Transformation behaviors and environmental risk assessment of heavy metals during resource recovery from Sedum plumbizincicola via hydrothermal liquefaction,” J. Hazard. Mater., vol. 410, May 2021, doi: 10.1016/j.jhazmat.2020.124588. en

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